globalchange  > 科学计划与规划
项目编号: NE/I020148/1
项目名称:
Aerosol-Cloud Interactions - A Directed Programme to Reduce Uncertainty in Forcing (ACID-PRUF) through a Targeted Laboratory and Modelling Programme
作者: Philip Stier
承担单位: University of Oxford
批准年: 2010
开始日期: 2011-13-12
结束日期: 2015-31-03
资助金额: GBP251823
资助来源: UK-NERC
项目类别: Research Grant
国家: UK
语种: 英语
特色学科分类: Climate & Climate Change&nbsp ; (70%) ; Geosciences&nbsp ; (20%) ; Pollution, waste & resources&nbsp ; (10%)
英文摘要: Aerosol particles act as sites for cloud droplet and ice particle formation. Cloud properties can be perturbed through the addition of aerosol particles into the atmosphere from anthropogenic and natural processes. This addition influences cloud microphysical properties, and subsequently affects cloud dynamics and thermodynamics, and the way the cloud interacts with radiation. The Earth's radiation budget is very greatly affected by clouds, and human-induced changes to the particle loading affecting them, known as indirect effects, are large and highly uncertain. A large part of this uncertainty is the result of poor knowledge of the fundamental aerosol and cloud properties and processes, leading to their poor representation in models. A programme of research is proposed here to i) directly investigate these processes in the laboratory, ii) evaluate the sensitivity of climate relevant parameters to the studied processes, iii) interpret the laboratory studies with detailed model investigations and iv) to incorporate and test new descriptions of the studied processes in cloud-scale and, where possible, global scale models. The programme will thereby reduce the uncertainty in estimates of radiative forcing and climate feedbacks relating to aerosol and cloud processes. The studies are split into those affecting warm clouds (those containing only liquid droplets) and those affecting clouds containing ice particles. The programme brings together an interdisciplinary team of researchers with expertise in 'warm' and 'cold' cloud and aerosol processes combining laboratory and multiscale modelling activities to deliver the improved predictive capability. The 'warm' laboratory work focuses on two major aspects i) the rate at which water is taken up by growing aerosol particles as they become cloud droplets (or 'activate) and ii) the ability of aerosol particles of various compositions to act as seeds for cloud droplets. These studies use a number of techniques including single particle optical levitation and investigations in a large photochemical chamber coupled to a large number of chemical and physical probes of ensembles of particles formed in simulated atmospheric chemical processes. The 'cold' work uses a similar coupling of a large, well-instrumented cloud chamber experiments and single particle levitation studies. The chambers used in both aspects will be coupled to investigate the impacts of aerosol transformation conditions on warm and cold cloud formation, using the instrumental payload from both chambers. A range of detailed models will be used to explicitly describe the processes by which aerosol particles interact with increasing relative humidity and reducing temperature to form cloud droplet and ice crystals and to their properties. The processes and properties will be represented in dynamical frameworks to predict the interactions between aerosols and clouds and their radiative effects at cloud resolving scales and radiative forcing of some of the investigated properties on global radiative forcing and feedbacks. The sensitivity of climate relevant parameters to the fundamental parameters investigated in the laboratory programme and their improved quantification will be evaluated using a simplified model 'emulator'.
资源类型: 项目
标识符: http://119.78.100.158/handle/2HF3EXSE/103298
Appears in Collections:科学计划与规划
气候变化与战略

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作者单位: University of Oxford

Recommended Citation:
Philip Stier. Aerosol-Cloud Interactions - A Directed Programme to Reduce Uncertainty in Forcing (ACID-PRUF) through a Targeted Laboratory and Modelling Programme. 2010-01-01.
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