globalchange  > 气候变化事实与影响
DOI: 10.1016/j.scitotenv.2018.10.217
WOS记录号: WOS:000454418500033
论文题名:
Identification, spatial extent and distribution of fugitive gas migration on the well pad scale
作者: Forde, O. N.1; Mayer, K. U.1; Hunkeler, D.2
通讯作者: Forde, O. N.
刊名: SCIENCE OF THE TOTAL ENVIRONMENT
ISSN: 0048-9697
EISSN: 1879-1026
出版年: 2019
卷: 652, 页码:356-366
语种: 英语
英文关键词: Natural gas ; Effluxes ; Stable carbon isotopes ; Hydraulic fracturing ; Gas migration ; Emissions
WOS关键词: METHANE EMISSIONS ; SHALE GAS ; ABANDONED OIL ; GROUNDWATER ; TRANSPORT ; LANDFILL ; ALBERTA ; QUANTIFICATION ; GEOCHEMISTRY ; SIGNATURES
WOS学科分类: Environmental Sciences
WOS研究方向: Environmental Sciences & Ecology
英文摘要:

Global methane (CH4) emissions are becoming increasingly important due to the contribution of CH4 to global warming. Leaking oil and gas wells can lead to subsurface CH4 gas migration (GM), which can cause both aquifer contamination and atmospheric emissions. Despite the need to identify and quantify GM at oil and gas well pads, effective and reliable monitoring techniques are lacking. In this field study, we used CH4 and carbon dioxide (CO2) efflux measurements together with soil gas stable carbon isotopic signatures to identify the occurrence and to characterize the spatio-temporal migration of fugitive gas across 17 selected well pads in Northeastern British Columbia, Canada. At 13 of these sites, operators had previously reported the occurrence of GM; however, subsequent inspections based on visual, olfactory or auditory evidence only identified GM at two of these sites. Using the soil gas efflux method, evidence for GM was found at 15 of the 17 well pads with CH4 and CO2 effluxes ranging from 0.017 to 180 mu mol m(-2) s(-1)(0.024 to 250 g CH4 m(-2) d(-1)) and 0.50 to 32 mu mol m(-2) s(-1) (1.9 to 122 g CO2 m(-2) d(-1)), respectively. Stable carbon isotopic composition was assessed at 10 of the 17 well pads with 9 well pads showing evidence of GM. The isotopic values indicated that CH4 in soil gas was from the same origin as CH4 in the surface casing vent flow gas. There was no correlation between CH4 effluxes and the distance from the well head; an equal portion of elevated effluxes were detected > 10 m from the well head as were detected < 5 m from the well head. In addition, CH4 effluxes varied temporally with values changing by up to an order of magnitude over 2 h. Although the study was carried out in Northeastern British Columbia, the results are applicable on a global scale, suggesting that inspections mostly based on visual evidence (e.g. bubbling at the well head) are not reliable for the identification of GM and, that infrequent survey measurements at predefined locations close to the well head may overestimate, underestimate or even miss CH4 effluxes. Repetitive and relatively densely spaced gas efflux measurements using a dynamic closed chamber method proved to be a useful tool for detecting GM. (C) 2018 Elsevier B.V. All rights reserved.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/130102
Appears in Collections:气候变化事实与影响

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作者单位: 1.Univ British Columbia, Dept Earth Ocean & Atmospher Sci, 2020-2007 Main Mall, Vancouver, BC V6T 1Z4, Canada
2.Univ Neuchatel, Fac Sci, Hydrogeol & Geothermal Ctr, CH-2000 Neuchatel, Switzerland

Recommended Citation:
Forde, O. N.,Mayer, K. U.,Hunkeler, D.. Identification, spatial extent and distribution of fugitive gas migration on the well pad scale[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019-01-01,652:356-366
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