globalchange  > 气候变化事实与影响
DOI: 10.3389/fpls.2019.00191
WOS记录号: WOS:000459370000002
论文题名:
Interannual and Seasonal Dynamics of Volatile Organic Compound Fluxes From the Boreal Forest Floor
作者: Maki, Mari1,2; Aalto, Juho1,3; Hellen, Heidi4; Pihlatie, Mari1,5,6; Back, Jaana1,2,6
通讯作者: Maki, Mari
刊名: FRONTIERS IN PLANT SCIENCE
ISSN: 1664-462X
出版年: 2019
卷: 10
语种: 英语
英文关键词: biogenic volatile organic compound ; flux ; forest floor ; temperature ; seasonality ; vegetation ; decomposition
WOS关键词: SCOTS PINE ; MONOTERPENE EMISSIONS ; ATMOSPHERIC OH ; CLIMATE-CHANGE ; VOC EMISSIONS ; PTR-TOF ; SOIL ; EXCHANGE ; MODEL ; METHANOL
WOS学科分类: Plant Sciences
WOS研究方向: Plant Sciences
英文摘要:

In the northern hemisphere, boreal forests are a major source of biogenic volatile organic compounds (BVOCs), which drive atmospheric processes and lead to cloud formation and changes in the Earth's radiation budget. Although forest vegetation is known to be a significant source of BVOCs, the role of soil and the forest floor, and especially interannual variations in fluxes, remains largely unknown due to a lack of long-term measurements. Our aim was to determine the interannual, seasonal and diurnal dynamics of boreal forest floor volatile organic compound (VOC) fluxes and to estimate how much they contribute to ecosystem VOC fluxes. We present here an 8-year data set of forest floor VOC fluxes, measured with three automated chambers connected to the quadrupole proton transfer reaction mass spectrometer (quadrupole PTR-MS). The exceptionally long data set shows that forest floor fluxes were dominated by monoterpenes and methanol, with relatively comparable emission rates between the years. Weekly mean monoterpene fluxes from the forest floor were highest in spring and in autumn (maximum 59 and 86 mu g m(-2) h(-1), respectively), whereas the oxygenated VOC fluxes such as methanol had highest weekly mean fluxes in spring and summer (maximum 24 and 79 mu g m(-2) h(-1), respectively). Although the chamber locations differed from each other in emission rates, the inter-annual dynamics were very similar and systematic. Accounting for this chamber location dependent variability, temperature and relative humidity, a mixed effects linear model was able to explain 79-88% of monoterpene, methanol, acetone, and acetaldehyde fluxes from the boreal forest floor. The boreal forest floor was a significant contributor in the forest stand fluxes, but its importance varies between seasons, being most important in autumn. The forest floor emitted 2-93% of monoterpene fluxes in spring and autumn and 1-72% of methanol fluxes in spring and early summer. The forest floor covered only a few percent of the forest stand fluxes in summer.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/130149
Appears in Collections:气候变化事实与影响

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作者单位: 1.Inst Atmospher & Earth Syst Res Forest Sci, Helsinki, Finland
2.Univ Helsinki, Fac Agr & Forestry, Dept Forest Sci, Helsinki, Finland
3.Univ Helsinki, Dept Phys, Fac Sci, Helsinki, Finland
4.Finnish Meteorol Inst, Helsinki, Finland
5.Univ Helsinki, Fac Agr & Forestry, Dept Agr Sci, Helsinki, Finland
6.Univ Helsinki, Viikki Plant Sci Ctr, Helsinki, Finland

Recommended Citation:
Maki, Mari,Aalto, Juho,Hellen, Heidi,et al. Interannual and Seasonal Dynamics of Volatile Organic Compound Fluxes From the Boreal Forest Floor[J]. FRONTIERS IN PLANT SCIENCE,2019-01-01,10
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