globalchange  > 气候变化事实与影响
DOI: 10.1126/sciadv.aav5077
WOS记录号: WOS:000466398400063
论文题名:
Calcium-looping reforming of methane realizes in situ CO2 utilization with improved energy efficiency
作者: Tian, Sicong1; Yan, Feng2,3; Zhang, Zuotai2; Jiang, Jianguo3
通讯作者: Tian, Sicong
刊名: SCIENCE ADVANCES
ISSN: 2375-2548
出版年: 2019
卷: 5, 期:4
语种: 英语
WOS关键词: SYNGAS PRODUCTION ; FLUIDIZED-BED ; CARBON ; CONVERSION ; CAPTURE ; CATALYSTS ; STEAM ; PERFORMANCE ; FEEDSTOCK ; SORBENTS
WOS学科分类: Multidisciplinary Sciences
WOS研究方向: Science & Technology - Other Topics
英文摘要:

Closing the anthropogenic carbon cycle is one important strategy to combat climate change, and requires the chemistry to effectively combine CO2 capture with its conversion. Here, we propose a novel in situ CO2 utilization concept, calcium-looping reforming of methane, to realize the capture and conversion of CO2 in one integrated chemical process. This process couples the calcium-looping CO2 capture and the CH4 dry reforming reactions in the CaO-Ni bifunctional sorbent-catalyst, where the CO2 captured by CaO is reduced in situ by CH4 to CO, a reaction catalyzed by catalyzed by the adjacent metallic Ni. The process coupling scheme exhibits excellent decarbonation kinetics by exploiting Le Chatelier's principle to shift reaction equilibrium through continuous conversion of CO2, and results in an energy consumption 22% lower than that of conventional CH4 dry reforming for CO2 utilization. The proposed CO2 utilization concept offers apromising option to recycle carbon directly at large CO2 stationary sources in an energy-efficient manner.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/133453
Appears in Collections:气候变化事实与影响

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作者单位: 1.Macquarie Univ, Sch Engn, Sydney, NSW 2109, Australia
2.Southern Univ Sci & Technol, Sch Environm Sci & Engn, Shenzhen 518055, Peoples R China
3.Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China

Recommended Citation:
Tian, Sicong,Yan, Feng,Zhang, Zuotai,et al. Calcium-looping reforming of methane realizes in situ CO2 utilization with improved energy efficiency[J]. SCIENCE ADVANCES,2019-01-01,5(4)
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