globalchange  > 气候变化事实与影响
DOI: 10.1021/acs.est.9b00596
WOS记录号: WOS:000463679600014
论文题名:
Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia
作者: Wu, Guangming1; Ram, Kirpa1,2; Fu, Pingqing3; Wang, Wan4; Zhang, Yanlin5; Liu, Xiaoyan5; Stone, Elizabeth A.6; Pradhan, Bidya Banmali7; Dangol, Pradeep Man7; Panday, Arnico K.7; Wan, Xin1,10; Bai, Zhipeng4; Kang, Shichang8,9; Zhang, Qianggong1,9; Cong, Zhiyuan1,9
通讯作者: Cong, Zhiyuan
刊名: ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN: 0013-936X
EISSN: 1520-5851
出版年: 2019
卷: 53, 期:7, 页码:3471-3479
语种: 英语
WOS关键词: LIGHT-ABSORPTION PROPERTIES ; CHEMICAL-COMPOSITION ; SOURCE APPORTIONMENT ; ORGANIC AEROSOLS ; BLACK CARBON ; BIOMASS ; FLUORESCENCE ; PM2.5 ; PM10 ; PARTICLES
WOS学科分类: Engineering, Environmental ; Environmental Sciences
WOS研究方向: Engineering ; Environmental Sciences & Ecology
英文摘要:

Brown carbon (BrC) has recently emerged as an important light-absorbing aerosol. This study provides interannual and seasonal variations in light absorption properties, chemical composition, and sources of water-soluble BrC (WS-BrC) based on PM10 samples collected in Godavari, Nepal, from April 2012 to May 2014. The mass absorption efficiency of WS-BrC at 365 nm (MAE(365)) shows a clear seasonal variability, with the highest MAE(365) of 1.05 +/- 0.21 m(2) g(-1) in premonsoon season and the lowest in monsoon season (0.59 +/- 0.16 m(2) g(-1)). The higher MAE(365) values in nonmonsoon seasons are associated with fresh biomass burning emissions. This is further substantiated by a strong correlation (r = 0.79, P < 0.01) between Abs(365) (light absorption coefficient at 365 nm) and levoglucosan. We found, using fluorescence techniques, that humic-like and protein-like substances are the main chromophores in WS-BrC and responsible for 80.2 +/- 4.1% and 19.8 +/- 4.1% of the total fluorescence intensity, respectively. BrC contributes to 8.78 +/- 3.74% of total light absorption over the 300-700 nm wavelength range. Considering the dominant contribution of biomass burning to BrC over Godavari, this study suggests that reduction in biomass burning emission may be a practical method for climate change mitigation in South Asia.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/134044
Appears in Collections:气候变化事实与影响

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作者单位: 1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
2.Banaras Hindu Univ, Inst Environm & Sustainable Dev, Varanasi 221005, Uttar Pradesh, India
3.Tianjin Univ, Inst Surface Earth Syst Sci, Tianjin 300072, Peoples R China
4.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
5.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Nanjing 210044, Jiangsu, Peoples R China
6.Univ Iowa, Dept Chem, Iowa City, IA 52246 USA
7.Int Ctr Integrated Mt Dev, Khumaltar 009771, Lalitpur, Nepal
8.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Gansu, Peoples R China
9.Chinese Acad Sci, Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
10.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Wu, Guangming,Ram, Kirpa,Fu, Pingqing,et al. Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2019-01-01,53(7):3471-3479
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