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DOI: 10.1016/j.ijhydene.2019.02.121
WOS记录号: WOS:000466618300019
论文题名:
Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems
作者: Marcantonio, Vera1; De Falco, Marcello2; Capocelli, Mauro2; Bocci, Enrico3; Colantoni, Andrea1; Villarini, Mauro1
通讯作者: Villarini, Mauro
刊名: INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
ISSN: 0360-3199
EISSN: 1879-3487
出版年: 2019
卷: 44, 期:21, 页码:10350-10360
语种: 英语
英文关键词: Biomass gasification ; Fluidized bed ; PSA ; Hydrogen production ; Quasi-equilibrium temperature ; Palladium membrane
WOS关键词: AIR-STEAM GASIFICATION ; MEMBRANE REACTORS ; CLIMATE-CHANGE ; SIMULATION ; POWER ; GAS ; PERFORMANCE ; PLANT ; FUEL ; SCALE
WOS学科分类: Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS研究方向: Chemistry ; Electrochemistry ; Energy & Fuels
英文摘要:

Gasification is one of the most effective and studied methods for producing energy and fuels from biomass as different biomass feedstock can be handled, with the generation of syngas consisting of H-2, CO, and CH4, which can be used for several applications. In this study, the gasification of hazelnut shells (biomass) within a circulating bubbling fluidized bed gasifier was analyzed for the first time through a quasi-equilibrium approach developed in the Aspen Plus environment and used to validate and improve an existing bubbling fluidized bed gasifier model. The gasification unit was integrated with a water-gas shift (WGS) reactor to increase the hydrogen content in the outlet stream and with a pressure swing adsorption (PSA) unit for hydrogen separation. The amount of dry H-2 obtained out of the gasifier was 31.3 mol%, and this value increased to 47.5 mol% after the WGS reaction. The simulation results were compared and validated against experimental data reported in the literature. The process model was then modified by replacing the PSA unit with a palladium membrane separation module. The final results of the present work allowed comparison of the effects of the two conditioning systems, PSA and palladium membrane, indicating a comparative increase in the hydrogen recovery ratio of 28.9% with the palladium membrane relative to the PSA configuration. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/136681
Appears in Collections:过去全球变化的重建

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作者单位: 1.Tuscia Univ Viterbo, Dept Agr & Forestry Sci DAFNE, Via San Camillo de Lellis Snc, I-01100 Viterbo, Italy
2.Univ Campus Bio Medico Roma, Dept Engn, Unit Proc Engn, Via Alvaro del Portillo 21, I-00128 Rome, Italy
3.Marconi Univ, Dept Nucl Subnucl & Radiat Phys, I-00193 Rome, Italy

Recommended Citation:
Marcantonio, Vera,De Falco, Marcello,Capocelli, Mauro,et al. Process analysis of hydrogen production from biomass gasification in fluidized bed reactor with different separation systems[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2019-01-01,44(21):10350-10360
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