globalchange  > 过去全球变化的重建
DOI: 10.1016/j.cplett.2019.02.041
WOS记录号: WOS:000462771900019
论文题名:
Atmospheric Chemistry of Methoxyflurane (CH3OCF2CHCl2): Kinetics of the gas-phase reactions with OH radicals, Cl atoms and O-3
作者: Hass, Sofie A.1; Andersen, Simone Thirstrup1; Andersen, Mads P. Sulbaek1,2; Nielsen, Ole J.1
通讯作者: Andersen, Mads P. Sulbaek
刊名: CHEMICAL PHYSICS LETTERS
ISSN: 0009-2614
EISSN: 1873-4448
出版年: 2019
卷: 722, 页码:119-123
语种: 英语
WOS关键词: RATE CONSTANTS ; ARRHENIUS PARAMETERS ; PHOTOCHEMICAL DATA ; HYDROXYL RADICALS ; CHLORINE ATOMS ; LIFETIMES ; CF3CHCLOCHF2 ; CF3CH2OCHF2 ; HYDROFLUOROETHERS ; CHF2OCF2CHFCL
WOS学科分类: Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS研究方向: Chemistry ; Physics
英文摘要:

Smog chamber techniques were used to determine k(CH3OCF2CHCl2 + Cl)=(5.04 +/- 0.75) x10(-13), k(CH3OCF2CHCl2 + OH)=(2.18 +/- 0.38) x10(-13), and k (CH3OCF2CHCl2 + O-3) < 1.5x10(-22) cm(3) molecule(-1) s(-1) in 700 Torr of N-2/air diluent at 296-300 K. The IR spectrum for CH3OCF2CHCl2 is reported. CH3OCF2CHCl2 is a short-lived compound with an estimated atmospheric lifetime of similar to 54 days. The ozone depletion potential for CH3OCF2CHCl2 was estimated to be on the order of 0.001 and a 100-year global warming potential of 4 was determined using a lifetime-corrected radiative efficiency estimation. Results are discussed with respect to the atmospheric chemistry of halogenated anesthetic gases.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/137056
Appears in Collections:过去全球变化的重建

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作者单位: 1.Univ Copenhagen, Dept Chem, Copenhagen Ctr Atmospher Res, Univ Parken 5, DK-2100 Copenhagen O, Denmark
2.Calif State Univ Northridge, Dept Chem & Biochem, Northridge, CA 91330 USA

Recommended Citation:
Hass, Sofie A.,Andersen, Simone Thirstrup,Andersen, Mads P. Sulbaek,et al. Atmospheric Chemistry of Methoxyflurane (CH3OCF2CHCl2): Kinetics of the gas-phase reactions with OH radicals, Cl atoms and O-3[J]. CHEMICAL PHYSICS LETTERS,2019-01-01,722:119-123
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