globalchange  > 全球变化的国际研究计划
DOI: 10.5194/acp-19-9663-2019
WOS记录号: WOS:000477971700004
论文题名:
Modeling the aging process of black carbon during atmospheric transport using a new approach: a case study in Beijing
作者: Zhang, Yuxuan1,2; Li, Meng2; Cheng, Yafang2; Geng, Guannan3; Hong, Chaopeng4; Li, Haiyan1; Li, Xin5; Tong, Dan4; Wu, Nana1; Zhang, Xin1; Zheng, Bo6; Zheng, Yixuan7; Bo, Yu1,8; Su, Hang2; Zhang, Qiang1
通讯作者: Bo, Yu ; Zhang, Qiang
刊名: ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN: 1680-7316
EISSN: 1680-7324
出版年: 2019
卷: 19, 期:14, 页码:9663-9680
语种: 英语
WOS关键词: AEROSOL OPTICAL-PROPERTIES ; PEARL RIVER-DELTA ; MIXING STATE ; ABSORPTION ENHANCEMENT ; PHYSICAL-PROPERTIES ; LIGHT-ABSORPTION ; SOURCE APPORTIONMENT ; HAZE POLLUTION ; BROWN CARBON ; SOOT
WOS学科分类: Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向: Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
英文摘要:

The effect of black carbon (BC) on air quality and the climate is still unclear, which is partly because of the poor understanding regarding the BC aging process in the atmosphere. In this work, we developed a new approach to simulate the BC mixing state (i.e., other species coated on the BC surface) based on an emissions inventory and back-trajectory analysis. The model tracks the evolution of the BC aging degree (characterized by the size ratio of the whole particle and BC core) during atmospheric transport. Using the models, we quantified the mass-averaged aging degree of total BC particles transported to a receptor (e.g., an observation site) from various emission origins (i.e., 0.25 degrees x 0.25 degrees grids). The simulations showed good agreement with the field measurements, which validated our model calculation. Modeling the aging process of BC during atmospheric transport showed that it was strongly dependent on emission levels. BC particles from extensive emission origins (i.e., polluted regions) were characterized by a higher aging degree during atmospheric transport due to more co-emitted coating precursors. On the other hand, high-emission regions also controlled the aging process of BC particles that were emitted from cleaner regions and passed through these polluted regions during atmospheric transport. The simulations identified the important roles of extensive emission regions in the BC aging process during atmospheric transport, implying the enhanced contributions of extensive emission regions to BC light absorption. This provides a new perspective on the phenomenon of pollution building up in the North China Plain, further demonstrating that this is mainly driven by regional transport and transformation. The simulation of the BC aging degree during atmospheric transport provided more clues for improving air pollution and climate change.


Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/143917
Appears in Collections:全球变化的国际研究计划

Files in This Item:

There are no files associated with this item.


作者单位: 1.Tsinghua Univ, Dept Earth Syst Sci, Beijing 100084, Peoples R China
2.Max Planck Inst Chem, Multiphase Chem Dept, D-55128 Mainz, Germany
3.Emory Univ, Rollins Sch Publ Hlth, Dept Environm Hlth, Atlanta, GA 30322 USA
4.Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA
5.Beijing Technol & Business Univ, Dept Environm Sci & Engn, Beijing 100048, Peoples R China
6.LSCE, Orme de Merisiers, Batiment 706,Pte 25, F-91191 Gif Sur Yvette, France
7.Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA
8.Chinese Acad Sci, Inst Atmospher Phys, RCE TEA, Beijing 100029, Peoples R China

Recommended Citation:
Zhang, Yuxuan,Li, Meng,Cheng, Yafang,et al. Modeling the aging process of black carbon during atmospheric transport using a new approach: a case study in Beijing[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019-01-01,19(14):9663-9680
Service
Recommend this item
Sava as my favorate item
Show this item's statistics
Export Endnote File
Google Scholar
Similar articles in Google Scholar
[Zhang, Yuxuan]'s Articles
[Li, Meng]'s Articles
[Cheng, Yafang]'s Articles
百度学术
Similar articles in Baidu Scholar
[Zhang, Yuxuan]'s Articles
[Li, Meng]'s Articles
[Cheng, Yafang]'s Articles
CSDL cross search
Similar articles in CSDL Cross Search
[Zhang, Yuxuan]‘s Articles
[Li, Meng]‘s Articles
[Cheng, Yafang]‘s Articles
Related Copyright Policies
Null
收藏/分享
所有评论 (0)
暂无评论
 

Items in IR are protected by copyright, with all rights reserved, unless otherwise indicated.