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Spatiotemporal patterns of evapotranspiration (ET) and its controlling factors are important for ecosystem services and water resources management in the Chinese Loess Plateau (CLP). In this study, we assessed the spatial patterns of ET and then investigated the interannual variability of ET and its relationships with climate variability and vegetation coverage changes at the timescales of annual, active growing season, as well as different seasons across the entire CLP from 2000 to 2014. A MODIS-derived ET dataset, ground-based datasets of precipitation and atmospheric evaporative demand (AED), and a remote-sensing dataset of Normalized Difference Vegetation Index (NDVI) were comprehensively analyzed. Results showed that mean annual ET varied distinctly among different vegetation zones, generally higher in the more humid southeastern parts of the CLP. Summer ET and ET over active growing season significantly increased for more than 40% of the entire CLP area, and winter ET significantly decreased over similar to 70% of the entire CLP region, while annual ET, spring ET, and autumn ET remained quite stable during 2000-2014. Per-pixel interannual variability of ET was mainly positively correlated with that of precipitation and NDVI except for winter, but negatively correlated with AED trends. Our study also demonstrated that ET variation trends were exactly consistent for the entire CLP region, the areas mainly implemented with the Grain for Green (GFG) project, and other CLP areas not implemented with the GFG project during 2000-2014. Our findings suggest that the spatiotemporal patterns of CLP ET were mainly water-limited, and climate variability played an essential role in shaping the interannual variability of ET in the CLP. This study will improve our understanding on the ET variations over water-limited areas under climate and vegetation coverage changes.