globalchange  > 气候变化与战略
CSCD记录号: CSCD:5744083
论文题名:
亚热带典型岩溶溪流水气界面CO_2交换通量变化过程及其环境影响
其他题名: Variations of CO_2 Exchange Fluxes Across Water-air Interface and Environmental Meaning in a Surface Stream in Subtropical Karst Area, SW China
作者: 李丽1; 蒲俊兵2; 李建鸿1; 于奭2; 肖琼2; 张陶1
刊名: 环境科学
ISSN: 0250-3301
出版年: 2016
卷: 37, 期:7, 页码:220-231
语种: 中文
中文关键词: 岩溶地表溪流 ; CO_2脱气 ; 通量 ; 影响因素 ; 官村岩溶地表溪流
英文关键词: karst surface stream ; CO_2 degassing ; fluxes ; influencing factors ; Guancun karst subterranean stream
WOS学科分类: ENVIRONMENTAL SCIENCES
WOS研究方向: Environmental Sciences & Ecology
中文摘要: 具有较高水体CO_2分压(pCO_2)的岩溶地下水出露地表后常与大气形成较高的正向CO_2浓度梯度,因此评价岩溶水体水气界面CO_2交换通量对于岩溶碳循环过程研究具有重要意义.本文以广西柳州官村地下河补给的地表溪流为研究对象,详细讨论了岩溶溪流水-气界面CO_2交换通量.使用静态箱法和手持式二氧化碳测量仪GM70对脱气通量进行检测,结果表明,溪流的CO_2交换通量以脱气为主,地下河出口(G1点)脱气通量变化范围为139.48~890.84 mg·(m~2·h)~(-1),平均值为445.72 mg·(m~2·h)~(-1),溪流下游(G2点)脱气通量变化范围为16.54~844.18 mg·(m~2·h)~(-1),平均值为159.81 mg·(m~2·h)~(-1),脱气通量的时空变化特征表现为雨季要大于旱季,地下河出口地区要大于下游地区.溪流CO_2脱气会对附近空气中CO_2气体碳同位素(delta~(13)C-CO_2)产生影响,使溪流附近空气中CO_2气体碳同位素(delta~(13)C-CO_2)值逐渐偏负,并表现出明显的时空变化,即delta~(13)C-CO_2雨季偏负于旱季,G1点delta~(13)C-CO_2偏负于G2点.并且由于脱气作用的进行,溪流的水化学性质沿流程变化,表现为HCO_3~-沿流程逐渐降低,pH值升高,电导率降低,pCO_2沿流程递减,常见碳酸盐矿物的饱和指数SIc逐渐升高,delta~(13)C-DIC值逐渐偏正.
英文摘要: CO_2 cycle process or sources/sinks are not only the basis of understanding and responding to global climate change, but also the core of the current global climate change research. Gas exchange across water-air interface in terrestrial surface water is an important way of nutrient elements (carbon, nitrogen) exchange between aquatic ecosystems and ambient air. Escaping CO_2 gas from surface water is also actively involved in the modern carbon cycle. In the material cycle in karst regions, CO_2 plays a key role in karst processes, driving the formation of karst features. Karst groundwater with high water CO_2 partial pressure (pCO_2) often shows highly positive CO_2 concentration gradient to atmosphere after it is discharged to surface, so the evaluation of CO_2 exchange fluxes across karst water-air interface is important for karst carbon cycle research. This paper researched CO_2 exchange fluxes across water-air interface in the karst surface stream in detail which was fed by Guancun subterranean stream in Liuzhou city, Guangxi province. Closed static chamber method and portable hand-holding CO_2 sensor (GM70) were both employed in CO_2 exchange fluxes monitoring. The results showed that CO_2 degassing was the mainly form of CO_2 exchange across the steam water-air interface. CO_2 degassing flux in subterranean stream outlet (G1 site) ranged from 139.48 to 890.84 mg·(m~2·h)~(-1) with an average of 445.72 mg·(m~2·h)~(-1). CO_2 degassing flux in stream downstream site (G2 site) ranged from 16.54 to 844.18 mg·(m~2·h)~(-1) with an average of 159.81 mg·(m~2·h)~(-1). The CO_2 degassing flux in G1site was higher than that in G2 site. CO_2 degassing fluxes in rainy season in both G1 and G2 site were higher than those in dry season. Stable carbon analysis of CO_2 gas (delta~(13)C-CO_2) found that CO_2 degassing from karst stream might influence air CO_2 carbon isotope near water surface, which resulted in the more negative delta~(13)C-CO_2 value with the increase of CO_2 degassing flux. Significant spatio-temporal variations of delta~(13)C-CO_2 were found, and the delta~(13)C-CO_2 in the rainy season was more negative than that in dry season and delta~(13)C-CO_2 in G1 site was more negative than that in G2 site. As a result of stream CO_2 degassing, the hydrochemical characteristics of steam varied along stream running, which resulted in decrease of HCO_3~-, EC and pCO_2 and increase of pH, SIc and delta~(13)C-DIC in the stream.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/150994
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作者单位: 1.西南大学地理科学学院, 重庆 400715, 中国
2.中国地质科学院岩溶地质研究所, 国土资源部、 广西岩溶动力学重点实验室, 桂林, 广西 541004, 中国

Recommended Citation:
李丽,蒲俊兵,李建鸿,等. 亚热带典型岩溶溪流水气界面CO_2交换通量变化过程及其环境影响[J]. 环境科学,2016-01-01,37(7):220-231
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