globalchange  > 气候变化与战略
CSCD记录号: CSCD:5643842
论文题名:
南极中山站大气六氟化硫浓度本底特征
其他题名: Background characteristics of atmospheric sulfur hexafluoride concentrations at Zhongshan Station, Antarctica
作者: 王灿1; 卞林根2; 叶文娟1; 朱仁斌1; 郑向东2; 刘立新2
刊名: 科学通报
ISSN: 0023-074X
出版年: 2016
卷: 61, 期:7, 页码:22-28
语种: 中文
中文关键词: 南极 ; 中山站 ; 六氟化硫浓度 ; 大气 ; 本底浓度
英文关键词: Antarctica ; Zhongshan Station ; SF_6 concentration ; atmosphere ; background concentration
WOS学科分类: MULTIDISCIPLINARY SCIENCES
WOS研究方向: Science & Technology - Other Topics
中文摘要: 六氟化硫(SF_6)是一种增温潜能极高、主要来自人为排放的温室气体, 对其大气背景浓度进行长期监测,对于研究全球变化具有重要意义. 利用南极中山站区2008年2月~2013年1月近5年SF_6浓度的观测资料, 对SF_6本底浓度和变化趋势进行了研究, 结果表明: 中山站风向为偏东风时大气中SF_6浓度较低, 风向为偏西风时浓度较高,这主要是受海陆气团差异引起, 而局地源和风速的影响可忽略不计. 大气SF_6浓度的变化范围为6.01~7.80 pptv (1 pptv=1*10~(-12) L/L, 下同), 平均浓度为6.900.40 pptv. SF_6浓度呈明显稳定的年增长趋势, 年平均增长速率为0.28 pptv a~(-1), 其变化趋势与全球其他观测点较接近, 中山站的观测结果可代表南极地区SF_6的本底浓度. 通过与全球其他观测点大气SF_6浓度数据对比, 结果显示: 南半球大气SF_6平均浓度明显低于北半球, 北半球是SF_6排放的主要源区; 而南半球SF_6主要来源于北半球大气传输和南北半球间大气高度混合, 能较好地反映全球大气SF_6本底浓度. 南极受人类活动影响很小, 是研究全球SF_6浓度变化趋势的理想区域.
英文摘要: Sulfur hexafluoride (SF_6) is one kind of highly stable anthropogenic greenhouse gas with a global warming potential (GWP) of 2.35*10~4 over a 100-year time horizon. SF_6 emissions are targeted for reduction under the Kyoto Protocol. Therefore it is important for the research about global change to observe atmospheric SF_6 background concentrations. Here, we present the patterns for the seasonal and annual variations of atmospheric SF_6 concentrations at Zhongshan Station, east Antarctica from February 2008 to January 2013. The prevailing wind direction at the observation site was from the east with the frequency of 92.0%. The average SF_6 concentration was about 6.89 pptv under east wind, lower than that under west wind (7.16 pptv). More frequent west wind occurred in autumn and thus average SF_6 concentration was higher in autumn than other seasons, indicating that the airflow from western sea area contained higher SF_6 concentration than the airflow from east Antarctic continent. On the whole, SF_6 concentrations showed an insignificant change under different wind speeds and directions, indicating that the influence of wind and local pollution could be ignored. Our results could represent the background concentrations for atmospheric SF_6 at Zhongshan Station. The SF_6 concentrations ranged from 6.01 to 7.80 pptv with the average of 6.900.40 pptv from February 2008 to January 2013. Annual SF_6 concentrations in the atmosphere steadily increased at the rate of 0.28 pptv a~(-1), and the increasing magnitudes were very close to each other per year during the period of 2008-2012, similar to the results from other global observation sites, indicating that annual SF_6 emission amount could be almost stable each year. No evident periodical changes in SF_6 concentrations were observed during the five years. The seasonal SF_6 concentration did not show insignificant variation in spring and summer, but an evident decrease in its level occurred in autumn, and then it rose back to normal level in winter. Combined our data with those from other nine observation sites, atmospheric SF_6 concentrations showed an evident gradient change with the latitudes at the global scale, and its concentrations in the Northern Hemisphere were 0.3-0.4 pptv higher than those in the Southern Hemisphere because the main emission sources for atmospheric SF_6 concentrated in the Northern Hemisphere. The primary source for atmospheric SF_6 is industrial emissions in the Northern Hemisphere, whereas its main source is the SF_6 southward transportation in the Southern Hemisphere. Our results prove that atmospheric SF_6 concentration is continuously growing and its industrial emission control needs to be strengthened. Antarctica is less affected by human activities on the globe, which makes it an ideal area to observe SF_6 background concentrations. Our data in the present study will guide industry in optimizing and controlling the SF_6 emissions. The SF_6 sources and its transportation pathways will be further studied at Zhongshan Station in the future.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/151048
Appears in Collections:气候变化与战略

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作者单位: 1.中国科学技术大学地球和空间科学学院极地环境研究室, 合肥, 安徽 230026, 中国
2.中国气象科学研究院, 北京 100081, 中国

Recommended Citation:
王灿,卞林根,叶文娟,等. 南极中山站大气六氟化硫浓度本底特征[J]. 科学通报,2016-01-01,61(7):22-28
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