globalchange  > 气候变化与战略
CSCD记录号: CSCD:5793742
论文题名:
汽油车尾气排放CO_2的稳定同位素特征
其他题名: Stable Isotopic Characteristics of CO_2 Emitted by Gasoline Vehicles
作者: 肖瑶1; 胡敏1; 李梦仁1; 秦艳红1; 彭剑飞1; 张文彬2; 郑竞1; 杜卓菲1; 邓磊2; 帅石金2
刊名: 中国电机工程学报
ISSN: 0258-8013
出版年: 2016
卷: 36, 期:16, 页码:2794-2807
语种: 中文
中文关键词: 汽油车 ; 二氧化碳 ; 稳定碳同位素特征 ; 同位素分馏 ; 碳排放
英文关键词: gasoline vehicles ; carbon dioxide ; stable carbon isotopic characteristics ; isotope fractionation ; carbon emission
WOS学科分类: ENVIRONMENTAL SCIENCES
WOS研究方向: Environmental Sciences & Ecology
中文摘要: 温室气体CO_2浓度增长引起的气候变化问题受到全球广泛关注。CO_2的稳定碳同位素特征可为其源汇机制研究提供有力支持,但需要各类污染源排放的碳同位素特征值,尤其是局地或区域特征作为数据基础。CO_2浓度的增长主要来自化石燃料燃烧,机动车排放是一个重要来源。研究应用基于激光的同位素比红外光谱仪(IRIS),对我国汽油车尾气排放CO_2的稳定碳同位素组成(delta ~(13)C)进行了初步的研究,测定结果为(-28.0 0.5)。汽油车尾气排放CO_2出现碳同位素分馏现象,其 delta ~(13)C特征受冷热起动方式影响不大,但与汽油成分、发动机燃烧模式等相关;汽油车尾气排放CO_2的 delta ~(18)O特征变化较大,同位素分馏更为复杂。化石燃料燃烧产生CO_2的 delta ~(13)C特征对化石燃料具有较好的指示作用。本研究为碳排放研究提供了重要的数据支持。
英文摘要: The Problem of climate change caused by the increase of greenhouse gas CO_2 concentration attracts the world's attention. Stable carbon isotopic characteristics of CO_2 can provide strong support for the study of source and sink mechanism of CO_2. However, this needs the stable carbon isotope composition of different emission sources, specially local or regional sources as data base. The combustion of fossil fuel contributes a lot to the increase of CO_2 concentration, especially the emission of vehicles. In this study, we used laser-based isotope ratio infrared spectrometer (IRIS) to measure the delta ~(13)C characteristics of CO_2 emitted by gasoline vehicles in China, getting its stable carbon isotope composition (delta ~(13)C) of (-28.0 0.5). Carbon isotope fractionation exists in CO_2 emitted by gasoline vehicles. delta ~(13)C of CO_2 emitted by gasoline vehicles is not affected by cold start or hot start basically, but the composition of gasoline and engine combustion mode can influence delta ~(13)C of CO_2. The delta ~(18)O characteristics of CO_2 emitted by gasoline vehicles changes a lot, with more complicated isotope fractionation. The delta ~(13)C characteristics of CO_2 from combustion processes of fossil fuels can be a good indicator for fossil fuels. The delta ~(13)C of CO_2 emitted by gasoline vehicles as representative of China can be obtained from this preliminary study, providing basic foundation for the carbon emissions research in China.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/151832
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作者单位: 1.北京大学, 环境模拟与污染控制国家重点联合实验室, 北京 100871, 中国
2.清华大学, 汽车安全与节能国家重点实验室, 北京 100084, 中国

Recommended Citation:
肖瑶,胡敏,李梦仁,等. 汽油车尾气排放CO_2的稳定同位素特征[J]. 中国电机工程学报,2016-01-01,36(16):2794-2807
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