globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:6110599
论文题名:
反式-1-氯-3,3,3-三氟丙烯的制备研究进展
其他题名: Progress of preparation of trans-1-chloro-3,3,3-trifluoropropene
作者: 曾纪珺; 韩升; 唐晓博; 赵波; 郝志军; 张伟; 吕剑
刊名: 化工进展
ISSN: 1000-6613
出版年: 2017
卷: 36, 期:11, 页码:35-40
语种: 中文
中文关键词: 反式-1-氯-3,3,3-三氟丙烯 ; 发泡剂 ; 合成 ; 分离
英文关键词: trans-1-chloro-3,3,3-trifluoropropene[HCFO-1233zd(E)] ; blowing agent ; synthesis ; separation
WOS学科分类: ENGINEERING CHEMICAL
WOS研究方向: Engineering
中文摘要: 反式-1-氯-3,3,3-三氟丙烯[HCFO-1233zd(E)]的臭氧消耗潜值(ODP)为0.00024,温室效应潜值(GWP)为7.0,环保性能优良,已被国际社会认定为第四代氟代烃发泡剂,应用前景广阔。本文对现有HCFO-1233zd(E)制备方法进行综述,通过比较各合成路线优缺点,提出以HCC-240fa及其衍生物为原料的合成路线最具工业化前景。同时,对制备工艺中涉及的HCFO-1233zd(E)与HF和副产物共沸分离问题进行了分析总结。最后指出高效的氟化催化剂和绿色的分离工艺是未来HCFO-1233zd(E)工业化开发的研究重点。
英文摘要: Trans-1-chloro-3,3,3-trifluoropropene [HCFO-1233zd(E)] has virtually zero ozone depletion potential(ODP,0.00024)and very low global warming potential(GWP,7),and therefore it has been proposed as the fourth-generation blowing agent to replace 1,1-dichloro-1-fluoroethane(HCFC-141b) and 1,1,1,3,3-pentafluoropropane(HFC-245fa),due to its very low impact for environment. Synthetic methods of HCFO-1233zd(E) were summarized according to the starting materials. Compared with other routes,the process using HCC-240fa and its derivatives as starting material features good yield and excellent selectivity,and thus has an industrialization prospect. Moreover,the azeotropic separation of HCFO-1233zd(E) with HF and by-product in the preparation process was analyzed and summarized. Developing efficient fluorination catalyst and environmentally friendly purification technology is fundamentally important for industrial synthesis of HCFO-1233zd(E).
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/152602
Appears in Collections:气候变化事实与影响

Files in This Item:

There are no files associated with this item.


作者单位: 西安近代化学研究所, 氟氮化工资源高效开发与利用国家重点实验室, 西安, 陕西 710065, 中国

Recommended Citation:
曾纪珺,韩升,唐晓博,等. 反式-1-氯-3,3,3-三氟丙烯的制备研究进展[J]. 化工进展,2017-01-01,36(11):35-40
Service
Recommend this item
Sava as my favorate item
Show this item's statistics
Export Endnote File
Google Scholar
Similar articles in Google Scholar
[曾纪珺]'s Articles
[韩升]'s Articles
[唐晓博]'s Articles
百度学术
Similar articles in Baidu Scholar
[曾纪珺]'s Articles
[韩升]'s Articles
[唐晓博]'s Articles
CSDL cross search
Similar articles in CSDL Cross Search
[曾纪珺]‘s Articles
[韩升]‘s Articles
[唐晓博]‘s Articles
Related Copyright Policies
Null
收藏/分享
所有评论 (0)
暂无评论
 

Items in IR are protected by copyright, with all rights reserved, unless otherwise indicated.