globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:5999215
论文题名:
1.572 mum附近CO_2吸收光谱的测量
其他题名: Measurement of absorption spectrum around 1.572 mum
作者: 邵君宜1; 林兆祥1; 刘林美1; 龚威2
刊名: 物理学报
ISSN: 1000-3290
出版年: 2017
卷: 66, 期:10, 页码:431-436
语种: 中文
中文关键词: 大气光学 ; 激光雷达 ; CO_2吸收光谱 ; 双光路差分
英文关键词: atmospheric optics ; lidar ; absorption spectrum of CO_2 ; the differential system of double optical path
WOS学科分类: OPTICS ; PHYSICS MULTIDISCIPLINARY
WOS研究方向: Optics ; Physics
中文摘要: 应用自行构建的恒温差分吸收光谱探测系统,在230-320 K的温度范围内,精确探测1.572 mum附近CO_2吸收谱线的变化,获得了不同温度和压强下CO_2气体的吸收截面、自增宽系数、空气增宽系数,这些参数补充和完善了现有的数据库.定量分析了温度、压强对谱线的影响,建立了光学厚度和吸收截面的数值计算模型,并已经用于我国的CO_2激光雷达,为其高精度数据反演奠定了技术基础.这些工作能够提高工作在该波段的差分吸收CO_2探测激光雷达的反演精度.
英文摘要: Differential absorption lidar (DIAL) is widely accepted as a most promising remote sensing technique for measuring the atmospheric CO_2,and has been built in many countries to study the global climate change and carbon cycle. However,the imperfect information about CO_2 spectrum leads to evident errors in estimating some parameters (such as the absorption cross sections,the broadening coefficients,the optical depth,etc.) which are the critical parameters in retrieving processes of a DIAL,and will eventually result in unacceptable errors of XCO_2 retrievals. Coping with that problem,a self-built constant temperature differential absorption spectroscopy system has been set up which can be used to accurately measure the absorption spectrum of carbon dioxide in the band of 1.57 mum.On that basis,the absorption spectra of the pure carbon dioxide are measured respectively at the temperatures from 230 K to 320 K and the pressures from 20 kPa to 100 kPa by the highprecision oscilloscope and wavelength meter. A series of optical depths at absorption peak is respectively calculated at different temperatures and the results show that the optical depth linearly and monotonically changes while the temperature increases from 230 K to 320 K. At the same time,the relations between the corresponding absorption cross sections and temperature are analyzed,showing that the absorption cross sections first increases and then decreases with temperature increasing. The self-broadening coefficients are inferred from the spectral data at the same temperature and different pressures,and the temperature-dependent exponent is calculated. Furthermore,the air-broadening coefficients are calculated by carbon dioxide absorption spectrum data from different mixing ratios and its temperature-dependent exponent is obtained. The temperature-dependent exponent of self-broadening coefficient is 0.644 and the temperature-dependent exponent of air-broadening coefficient is 0.764,which are almost the same as the data in the high-resolution transmission molecular absorption database (HITRAN). The numerical calculation formulae of optical depth and absorption cross section are verified through these results.Those parameters supplement the widely-used HITRAN database. Moreover,quantitative analysis is conducted to explore the influences of temperature and pressure on CO_2 spectrum,thereby establishing a function for modeling the differential absorption optical depth and the absorption cross-section. The above results have already been used in China's CO_2-DIAL and lay a foundation of accurate retrieval. It is believed that other similar CO_2-DIAL of which operating wavelength is around 1.572 mum would also benefit from those newly measured parameters.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/153245
Appears in Collections:气候变化事实与影响

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作者单位: 1.中南民族大学电子信息工程学院, 武汉, 湖北 430074, 中国
2.武汉大学, 测绘遥感信息工程国家重点实验室, 武汉, 湖北 430079, 中国

Recommended Citation:
邵君宜,林兆祥,刘林美,等. 1.572 mum附近CO_2吸收光谱的测量[J]. 物理学报,2017-01-01,66(10):431-436
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