globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:6223577
论文题名:
2015年秋冬季武汉城区黑碳气溶胶的分布及源区分析
其他题名: The Analysis of Distribution and Source Area of Black Carbon Aerosol in Wuhan City in Autumn and Winter of 2015
作者: 黄超1; 赵锦慧1; 何超2; 刘玉青1; 李小莉1; 刘书凯3
刊名: 生态环境学报
ISSN: 1674-5906
出版年: 2018
卷: 27, 期:3, 页码:636-643
语种: 中文
中文关键词: 黑碳气溶胶 ; 时空分布 ; 相关性分析 ; 武汉 ; 多元线性回归分析 ; 轨迹模型
英文关键词: black carbon aerosol ; the temporal and spatial distribution ; correlation analysis ; Wuhan ; multiple linear regression analysis ; trajectory model
WOS学科分类: ENVIRONMENTAL SCIENCES
WOS研究方向: Environmental Sciences & Ecology
中文摘要: 黑碳(Black Carbon,BC)作为大气气溶胶的重要组成部分,因其在太阳辐射平衡、气候变化等方面具有巨大作用,而受到广泛的关注与研究.利用2015年9月2016年2月10个城区公园绿地黑碳气溶胶观测数据以及同期空气污染物数据,运用相关性分析、多元线性回归分析、HYSPLIT4模型等方法,分析了武汉市黑碳气溶胶的时空分布规律及其与空气污染物的关系,将BC本底浓度与各城市进行对比,并对两次较大规模的BC污染事件进行后向轨迹模拟.结果如下,(1)武汉市秋冬季BC质量浓度日均值为(5.2273.12) mug·m~(-3),范围为1.205~16.534 mug·m~(-3).(2)BC质量浓度在月变化上呈1月>12月>2月>10月>9月>11月,冬季整体高于秋季.(3)BC质量浓度最高值出现在石门峰公园,最低值出现在东湖风景区,导致空间分布差异的原因是离车流较多的主路距离不同.(4)采用最大频数法计算得到武汉市秋冬季黑碳气溶胶本底浓度为5.45 mug·m~(-3),与西宁、乌鲁木齐、芝加哥等城市差异明显.(5)BC与PM_(10)、CO、O_3、PM_(2.5)的相关系数分别为0.658、0.8、-0.436、0.885,通过建立多元线性回归模型,得到回归方程Y=-1 136.564+4.216X_1+66.316X_2-7X_3+40.324X_4.(6)运用HYSPLIT4模型进行72 h后向轨迹模拟,结果表明两次较大规模的BC污染事件污染源不同.秋冬季的轨迹分析也说明武汉受到不同起源的空气气团影响.该研究可为武汉城区黑碳气溶胶观测提供数据资料,有助于推动中国黑碳气溶胶的系统观测研究工作.
英文摘要: As an important component of atmospheric aerosol, black carbon has been widely concerned and studied due to its tremendous role in solar radiation forcing and climate change. In order to study the distribution and environmental effect of black carbon aerosol in Wuhan city, based on the data of black carbon aerosol that observed from 10 parks' green lands of Wuhan city and the data of main pollutants from September 2015 to February 2016, the temporal and spatial distribution of BC aerosol during autumn and winter in Wuhan, its relationship with main pollutants, and the backward trajectory simulation of two large BC pollution events, were analyzed mainly by using correlation analysis, multiple linear regression analysis, and HYSPLIT4 model. At the same time, the concentrations of BC in Wuhan were compared with other major cities at home and abroad during autumn and winter. The results mainly included: (1) The daily average concentration of BC was (5.2273.12) mug·m~(-3), ranging from 1.205 to 16.534 mug·m~(-3). (2) The monthly average concentration of BC had a trend, which was January>December>September>September> November, and the BC concentration was higher in winter. (3) Shimenfeng Park was highest in ten parks, while East Lake Scenic spot was lowest in the spatial distribution of BC concentration variation, the main reason for this diversities was the close distance from factories that emit pollutants and main road. (4) The BC background concentration of Wuhan in autumn and winter was 5.45 mug·m~(-3) which was calculated by the maximum frequency method. It had a difference obviously with Xining, Chicago, Urumqi, etc. (5) BC had a negative correlation with O_3 and positively correlated with PM_(2.5), PM_(10), CO, the correlation coefficients respectively were-0.436, 0.885, 0.658, and 0.8. By using multiple linear regression model, its regression equation came as follow: Y=-1 136.564+4.216X_1 +66.316X_2-7X_3+40.324X_4. And (6) the two large BC pollution events were analyzed by back-trajectory model. It indicated that the two sources of pollution were different. And the trajectory analysis of different seasons also showed that Wuhan was affected by different air masses in the autumn and winter. The research results can provide data foundation for black carbon aerosol observation in Wuhan city, and improve the systematic observation and research of black carbon aerosol in China.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/154577
Appears in Collections:气候变化事实与影响

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作者单位: 1.湖北大学资源环境学院, 武汉, 湖北 430062, 中国
2.武汉大学资源与环境科学学院, 武汉, 湖北 430072, 中国
3.西南林业大学国家高原湿地研究中心, 昆明, 云南 650224, 中国

Recommended Citation:
黄超,赵锦慧,何超,等. 2015年秋冬季武汉城区黑碳气溶胶的分布及源区分析[J]. 生态环境学报,2018-01-01,27(3):636-643
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