globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:6537709
论文题名:
基于TiO_2表面紫外光催化降解高浓度SF_6的实验与仿真研究
其他题名: Simulation and Experimental Study on Degradation of High Concentration SF_6 Based on Ultraviolet Photocatalysis Principle of Titanium Dioxide Surface
作者: 张晓星1; 李亚龙2; 胡雄雄3; 肖焓艳3; 崔兆仑2; 陈达畅2
刊名: 高电压技术
ISSN: 1003-6520
出版年: 2019
卷: 45, 期:7, 页码:840-846
语种: 中文
中文关键词: 降解率 ; 紫外光 ; 催化剂 ; 表面吸附
英文关键词: SF_6 ; TiO_2 ; SF_6 ; degradation rate ; TiO_2 ; ultraviolet ; catalyst ; surface adsorption
WOS学科分类: CHEMISTRY PHYSICAL
WOS研究方向: Chemistry
中文摘要: SF_6具有较高的温室效应潜在值(global warming potential,GWP),未经处理排放到大气中会对环境产生影响。电力工业中SF_6的应用越来越广泛,废气排放量也高速增长。为减少电力工业中SF_6废气对环境的污染,基于TiO_2表面在紫外光照射下具有催化效应这一特性,设计了一套实验平台,研究了不同数量的TiO_2催化剂和有 H_2O参与时对常温常压下高浓度SF_6降解效果的影响,并通过仿真分析了SF_6气体分子在TiO_2表面的断键分解过程。研究结果表明:TiO_2作为催化剂能够有效提高SF_6的降解率。其中,未加TiO_2时SF_6在紫外光照3 h后的降解率仅为1.25%,加入8个TiO_2片时相同条件下3 h降解率达到8.98%,降解产物主要有SO_2F_2、SiF_4、SF_4以及 SO_2;在此基础上,在SF_6气体中混入H_2O能把降解率提高到27.22%,降解产物主要有SO_2F_2、SiF_4、SF_4、SiH_4、 HF和SO_2。仿真计算结果表明TiO_2催化降解SF_6过程是把所需的能量细分为几个小的能量吸收过程,从能量吸收的角度解释了TiO_2催化降解SF_6的优势。研究结果可为SF_6的降解提供参考。
英文摘要: SF_6 has a high global warming potential (GWP),and will be harmful to the environment if the SF_6 is discharged into the atmosphere without treatment.The SF_6 is more extensively applied in the power industry and the exhaust emissions are also increasing rapidly.In order to reduce the environmental pollution of SF_6 exhaust gas in power industry,we designed a set of experimental platform based on the catalytic effect of TiO_2 surface under ultraviolet irradiation to study the effects of different amounts of TiO_2 and H_2O participation on the degradation of high concentrations of SF_6 at normal temperature and pressure.At the same time,the process of catalytic decomposition of SF_6 gas molecule on TiO_2 surface was analyzed by simulation.The results show that TiO_2,as a catalyst,can effectively increase the degradation rate of SF_6.The degradation rate of SF_6 after ultraviolet irradiation for 3 hours in the absence of TiO_2 was only 1.25% and the degradation rate reached 8.98% with 8 pieces of TiO_2 added,and the main degradation products were SO_2F_2,SiF_4,SF_4,and SO_2.Besides,H_2O addition in SF_6 gas can increase the degradation rate to 27.22%.The main degradation products are SO_2F_2,SiF_4,SF_4,SiH_4,HF,and SO_2.The simulation calculation results show that the TiO_2 catalytic degradation of SF_6 is to subdivide the required energy into several small energy absorption processes which explains the advantages of TiO_2 catalytic degradation of SF_6 from the perspective of energy absorption.The study can provide a reference for the degradation of SF_6.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/155744
Appears in Collections:气候变化事实与影响

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作者单位: 1.武汉大学电气与自动化学院
2.重庆大学,
3.输配电装备及系统安全与新技术国家重点实验室, 武汉
4.,
5.重庆 430072
6.400044
7.武汉大学电气与自动化学院, 武汉, 湖北 430072, 中国
8.重庆大学, 输配电装备及系统安全与新技术国家重点实验室, 重庆 400044, 中国

Recommended Citation:
张晓星,李亚龙,胡雄雄,等. 基于TiO_2表面紫外光催化降解高浓度SF_6的实验与仿真研究[J]. 高电压技术,2019-01-01,45(7):840-846
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