globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:6433385
论文题名:
HKUST-1的制备及其在化学固定二氧化碳中的应用
其他题名: Synthesis of HKUST-1 and application in chemically fixed carbon dioxide
作者: 欧沙; 杨昌云; 王茜
刊名: 化学研究与应用
ISSN: 1004-1656
出版年: 2019
卷: 31, 期:2, 页码:85-95
语种: 中文
中文关键词: 金属-有机框架材料 ; 化学固定二氧化碳 ; 催化
英文关键词: metal-organic framework ; chemical fixation and conversion of CO_2 ; catalysis
WOS学科分类: CHEMISTRY PHYSICAL
WOS研究方向: Chemistry
中文摘要: 二氧化碳作为主要温室气体,引发了温室效应和一系列环境问题。为了减少二氧化碳排放并保持碳循环的平衡,通过化学固定将二氧化碳转化为增值产品的方法引起了人们的广泛关注。新兴的金属-有机骨架(MOFs)具有高表面积和均匀分散的催化位点,被认为是CO_2捕获和固定的理想的多相催化剂。本文研究了在温和反应条件(1atm CO_2和35℃)下,四丁基溴化铵作为助催化剂,HKUST-1催化环氧乙基苯与二氧化碳偶联反应的催化性能。HKUST-1显示出高效催化氧化苯乙烯环加成反应的活性,反应48 h后转化率可达88%。
英文摘要: Carbon dioxide(CO_2) , as the major greenhouse gas,had shown its powerful impact on global warming and a series of environmental issues.To eliminate the CO_2 emission and retain the balance of carbon cycle, the conversion of CO_2 into value added products via chemical fixation methods had attracted booming interests.The emerging metal-organic frameworks(MOFs) possessing high surface area and uniform dispersed catalytic sites had been considered the powerful heterogeneous catalysts for CO_2 capture and sequential fixation.In this work, the catalytic properties of the metal-organic framework HKUST-1 in cycloaddition of CO_2 to epoxides to produce cyclic carbonates with tetrabutylammonium bromide as co-catalyst at ambient reaction condition(1 atm CO_2 and 35 ℃) were investigated. After reaction for 48 hours,HKUST-1 demonstrated efficient catalytic activity for cycloaddtion of styrene oxide with a yield of 88%over 48 hours.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/155830
Appears in Collections:气候变化事实与影响

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作者单位: 贵州医科大学生物与工程学院, 贵阳, 贵州 550000, 中国

Recommended Citation:
欧沙,杨昌云,王茜. HKUST-1的制备及其在化学固定二氧化碳中的应用[J]. 化学研究与应用,2019-01-01,31(2):85-95
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