DOI: 10.1073/pnas.1719443115
论文题名: Multidimensional photon correlation spectroscopy of cavity polaritons
作者: Dorfman K.E. ; Mukamel S.
刊名: Proceedings of the National Academy of Sciences of the United States of America
ISSN: 0027-8424
出版年: 2018
卷: 115, 期: 7 起始页码: 1451
结束页码: 1456
语种: 英语
英文关键词: Cavity polaritons
; Multidimensional spectroscopy
; Photon correlation
Scopus关键词: analytic method
; Article
; cavity polariton
; controlled study
; gated single photon emission computed tomography
; oscillation
; photobiology
; photochemistry
; photon correlation spectroscopy
; physical phenomena
; prediction
; priority journal
; scanning tunneling microscopy
; single photon emission computed tomography
; article
; cross coupling reaction
; energy transfer
; optical spectroscopy
; radiation field
英文摘要: The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes–Cummings model. © 2018 National Academy of Sciences. All Rights Reserved. Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/163743
Appears in Collections: 气候变化与战略
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作者单位: Dorfman, K.E., State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai, 200062, China; Mukamel, S., Department of Chemistry, University of California, Irvine, CA 92697, United States, Department of Physics and Astronomy, University of California, Irvine, CA 92697, United States
Recommended Citation:
Dorfman K.E.,Mukamel S.. Multidimensional photon correlation spectroscopy of cavity polaritons[J]. Proceedings of the National Academy of Sciences of the United States of America,2018-01-01,115(7)