英文摘要: | To have a >50% chance of limiting warming below 2 °C, most recent scenarios from integrated assessment models (IAMs) require large-scale deployment of negative emissions technologies (NETs). These are technologies that result in the net removal of greenhouse gases from the atmosphere. We quantify potential global impacts of the different NETs on various factors (such as land, greenhouse gas emissions, water, albedo, nutrients and energy) to determine the biophysical limits to, and economic costs of, their widespread application. Resource implications vary between technologies and need to be satisfactorily addressed if NETs are to have a significant role in achieving climate goals.
Despite two decades of effort to curb emissions of CO2 and other greenhouse gases (GHGs), emissions grew faster during the 2000s than in the 1990s1, and by 2010 had reached ~50 Gt CO2 equivalent (CO2eq) yr−1 (refs 2,3). The continuing rise in emissions is a growing challenge for meeting the international goal of limiting warming to less than 2 °C relative to the pre-industrial era, particularly without stringent climate policies to decrease emissions in the near future2, 3, 4. As negative emissions technologies (NETs) seem ever more necessary3, 5, 6, 7, 8, 9, 10, society needs to be informed of the potential risks and opportunities afforded by all mitigation options, to be able to decide which pathways are most desirable for dealing with climate change. There are distinct classes of NETs, such as: (1) bioenergy with carbon capture and storage (BECCS)11, 12; (2) direct air capture of CO2 from ambient air by engineered chemical reactions (DAC)13, 14; (3) enhanced weathering of minerals (EW)15, where natural weathering to remove CO2 from the atmosphere is accelerated and the products stored in soils, or buried in land or deep ocean16, 17, 18, 19; (4) afforestation and reforestation (AR) to fix atmospheric carbon in biomass and soils20, 21, 22; (5) manipulation of carbon uptake by the ocean, either biologically (that is, by fertilizing nutrient-limited areas23, 24) or chemically (that is, by enhancing alkalinity25); (6) altered agricultural practices, such as increased carbon storage in soils26, 27, 28; and (7) converting biomass to recalcitrant biochar, for use as a soil amendment29. In this Review, we focus on BECCS, DAC, EW and AR, because there are large uncertainties with ocean-based strategies (for example, ocean iron fertilization30), and other land-based approaches (for example, soil carbon and biochar storage) have been evaluated elsewhere31, 32, 33. Figure 1 depicts the main flows of carbon among atmospheric, land, ocean and geological reservoirs for fossil fuel combustion (Fig. 1a), bioenergy (Fig. 1b), carbon capture and storage (CCS; Fig. 1c) and the altered carbon flows entailed by each NET (Fig. 1d–h) when carbon is removed from the atmosphere.
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