globalchange  > 气候变化事实与影响
DOI: doi:10.1038/nclimate2804
论文题名:
Estimates of solid waste disposal rates and reduction targets for landfill gas emissions
作者: Jon T. Powell
刊名: Nature Climate Change
ISSN: 1758-763X
EISSN: 1758-6883
出版年: 2015-09-21
卷: Volume:6, 页码:Pages:162;165 (2016)
语种: 英语
英文关键词: Climate-change mitigation ; Environmental monitoring ; Sustainability
英文摘要:

Landfill disposal of municipal solid waste represents one of the largest anthropogenic global methane emission sources1, and recent policy approaches have targeted significant reductions of these emissions to combat climate change in the US (ref. 2). The efficacy of active gas collection systems in the US was examined by analysing performance data, including fire occurrence, from more than 850 landfills. A generalized linear model showed that the operating status of a landfill—open and actively receiving waste or closed—was the most significant predictor of collection system performance. Gas collection systems at closed landfills were statistically significantly more efficient (p < 0.001) and on average 17 percentage points more efficient than those at open landfills, but open landfills were found to represent 91% of all landfill methane emissions. These results demonstrate the clear need to target open landfills to achieve significant near-term methane emission reductions. This observation is underscored by landfill disposal rates in the US significantly exceeding previously reported national estimates, with this study reporting 262 million tonnes in the year 2012 compared with 122 million tonnes in 2012 as estimated by the US Environmental Protection Agency3.

The decomposition of municipal waste in landfills is recognized as one of the largest sources of global anthropogenic methane emissions1. Landfills represent the third-largest anthropogenic source of methane in the US, comprising approximately 18% of domestic emissions4. As such, the capture and combustion of landfill methane has been identified as a critical and viable near-term strategy for greenhouse gas (GHG) reductions associated with the waste sector5 in light of the cost and complexity of implementing wide-scale recycling and waste reduction efforts5. This is a particularly relevant strategy in lower- and lower–middle-income developing nations where waste generation is expected to increase 185% and 158%, respectively, over current rates by 2025 (ref. 6).

Although the US and many EU nations have required active landfill gas (LFG) capture for more than a decade7, 8, extensive data demonstrating the efficacy of these systems are limited. To fill this important gap, a new data set with more than 1,200 municipal solid waste landfills, both open and closed, resulting from the recently promulgated US GHG Reporting Rule9, 10 was analysed. The GHG reporting program requires municipal landfills that emit more than 25,000 tonnes of carbon dioxide equivalents to electronically report a substantial amount of operating data to the US Environmental Protection Agency (US EPA) annually, including: measured waste acceptance rates, locational data, projected disposal lifetime, and operational data for active gas collection systems (for example, total operational hours, collected methane content)11, if present. In addition, the GHG reporting rule sets out uniform procedures stipulating how sites must collect, validate and report these data.

Our analysis of this data set revealed that the total amount of municipal waste disposed of in the US was 262 million tonnes in 2012, 115% greater than the US EPA disposal estimate for the year 2012 (122 million tonnes) that used a materials flow analysis (top-down) approach3 and exceeds the World Banks projected municipal waste generation rate for the US in 2025 (ref. 6) of 256 million tonnes by about 4% (Fig. 1). Previously published survey estimates suggested that the US EPA disposal estimate was low12, but the facility-level nature of our estimate combined with the embedded quality assurance checks makes our estimate the most accurate for the US so far. As our estimate captures disposal at facilities subject to the GHG Reporting Rule, the quantities in Fig. 1 are likely to be underestimates because smaller landfills are not required to report. We estimated that an additional 10 million to 36 million tonnes of waste were disposed of in 2011 (see Supplementary Information). The differences in our estimate from the published top-down estimates are likely to stem from errors introduced in top-down methods associated with assumptions regarding waste generation factors for different economic indicators.

Figure 1: Quantity of municipal solid waste disposed of in US landfills.
Quantity of municipal solid waste disposed of in US landfills.

This study calculated the ‘GHG Reporting Data columns. Reported US EPA (2014) data3 were calculated using a materials flow analysis approach that calculates the disposal quantity on the basis of US census data and waste factors for industrial activity. US EPA data for the year 2013 were not available.

US EPA GHG Reporting Data.

Multiple queries were made through the US EPAs GHG Reporting Tool website (http://www.epa.gov/enviro/facts/ghg/customized.html) to source the municipal waste disposal quantity, LFG emissions, and LFG collection system performance data and metadata for reporting years 2010, 2011, 2012 and 2013. Every reporting landfill has a unique identification number, so data from the multiple queries were concatenated to develop a complete disposal and emissions profile for every open and closed landfill subject to the reporting rule. The total annual disposal quantity was calculated by summing the individually reported disposal quantities for every site in each reporting year. A generalized linear model was developed to identify significant predictors of LFG collection efficiency, including site operating status (open and actively receiving waste or closed), total methane generation, surface area containing waste, total landfill disposal capacity, number of gas collection wells installed, and measured methane concentration. Landfill operating status (open or closed) was found to be a significant (p < 0.05) predictor with limited residuals and no interaction with the variables that comprise the calculation of LFG collection efficiency. LFG collection efficiencies were analysed by first grouping open and closed landfills separately. The mean and 95% confidence interval of the mean collection efficiency were calculated in GraphPad Prism 6 (La Jolla). Statistical significance of LFG collection efficiency differences comparing open and closed landfills was calculated using two-sample t-tests in Minitab statistical software (State College). In a similar fashion, the significance of recirculating leachate at landfills on LFG collection efficiency was examined by conducting two-sample t-tests comparing sites that do and do not recirculate leachate frequently.

Methane emissions were calculated using a combination of data measured at each facility and modelled data—details of the equations used to determine methane emissions are presented in the Supplementary Information. Briefly, the emissions are computed using the amount of methane generated (modelled), the quantity of LFG collected (measured), the methane content of collected gas (measured), and the LFG collection efficiency (described previously). Although some uncertainty can be introduced when modelling LFG generation, the GHG Reporting Rule permits each facility to tailor LFG generation estimates according to the specific nature of the waste materials disposed of, if known, which results in greater model accuracy29.

Reported fire incidents at US municipal landfills.

US fire incident data were extracted from electronic databases provided by the National Fire Incident Reporting System (NFIRS), which reflects approximately 75% of all fire incidents in the US and represents fires electronically reported by fire departments across the US. Separate databases were provided to us by NFIRS for each year from 2004 to 2010. These data were compared with data from the US EPAs GHG Reporting data for the year 2010. Incidents specific to landfill fires were extracted from each year of the NFIRS data by isolating by incident type for ‘sanitary landfills (Code 152 in the database). Duplicate entries reflecting cases where more than one fire department responded to the same fire incident (corresponding to a ‘help code of 3 or 4 in the database) were removed. Annual fire frequency analysis was conducted in Microsoft Excel by creating a counting function for all fire incidents occurring in the same city. Identified repeat fire incidents at a single site were further analysed and incidents within the same city that occurred at a different address and at a location greater than 5 miles apart (as analysed using Google Maps Engine) were treated as separate fire incidents. Landfills with reported fire incidents were matched with landfills in the US EPA GHG Reporting database by matching the name and city (where available) of the site in each respective database. In limited cases, sites of the same name had mismatching cities, in which case the reported cities were mapped and those located within 5 miles of one another were considered to be the same site.

Additional analyses and corresponding methods related to the GHG Reporting data set and the NFIRS database are provided in the Supplementary Information.

  1. IPCC in Climate Change 2013: The Physical Science Basis (eds Stocker, T. F. et al.) (Cambridge Univ. Press, 2013).
  2. Davenport, C. White house unveils plans to cut methane emissions. New York Times (28 March 2014).
  3. Municipal Solid Waste Generation, Recycling, and Disposal in the United States: Facts and Figures 2012 (US EPA, 2014).
  4. Greenhouse Gas Sources and Sinks 1990–2011 (US EPA, 2013).
  5. van Renssen, S. Cleaning up rubbish. Nature Clim. Change 1, 439440 (2011).
  6. What a Waste: A Global Review of Solid Waste Management (World Bank, 2012).
  7. Proposed Rule—New Source Performance Standards (US EPA, 2014).
  8. Standards of Performance for Municipal Solid Waste Landfills; Proposed Rule 41796-41843 (Federal Register, 2014)
  9. National Fire Incident Reporting System Data: 2004–2010 (US Fire Administration, 2014)
  10. Envirofacts—Greenhouse Gas (US EPA, 2014).
  11. Mandatory Greenhouse Gas Reporting Vol. 40 (Code of Federal Regulations, 2010).
  12. van Haaren, R., Themelis, N. & Goldstein, N. The state of garbage in America. Biocycle 51, 1623 (2010).
  13. Spokas, K. et al. Methane mass balance at three landfill sites: What is the efficiency of capture by gas collection systems? Waste Manag. 26, 516525 (2006).
  14. Lohila, A. et al. Micrometeorological measurements of methane and carbon dioxide fluxes at a municipal landfill. Environ. Sci. Technol. 41, 27172722 (2007).
  15. Wang, X., Nagpure, A. S., DeCarolis, J. F. & Barlaz, M. A. Characterization of uncertainty in estimation of methane collection from select US landfills. Environ. Sci. Technol. 49, 15451551 (2015).
  16. Reinhart, D. R., McCreanor, P. T. & Townsend, T. The bioreactor landfill: Its status and future. Waste Manag. Res. 20, 172186 (2002).
  17. Wiedinmyer, C., Yokelson, R. J. & Gullett, B. K. Global emissions of trace gases, particulate matter, and hazardous air pollutants from open burning of domestic waste. Environ. Sci. Technol. 48, 95239530 (2014).
  18. Powell, J., Jain, P., Kim, H., Townsend, T. & Reinhart, D. Changes in landfill gas quality as a result of controlled air injection. Environ. Sci. Technol. 40, 6 (2006).
  19. Ruokojarvi, P., Ettala, M., Rahkonen, P., Tarhanen, J. & Ruuskanen, J. Polychlorinated Dibenzo-Dioxins and –Furans (PCDDs and PCDFs) in municipal waste landfill fires. Chemosphere 30, 16971708 (1995).
  20. El-Fadel, M., Findikakis, A. N. & Leckie, J. O. Environmental impacts of solid waste landfilling. J. Environ. Manag. 50, 125 (1997). URL:
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/4591
Appears in Collections:气候变化事实与影响
科学计划与规划
气候变化与战略

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Jon T. Powell. Estimates of solid waste disposal rates and reduction targets for landfill gas emissions[J]. Nature Climate Change,2015-09-21,Volume:6:Pages:162;165 (2016).
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