DOI: 10.1016/j.jcou.2015.07.002
Scopus记录号: 2-s2.0-84948098665
论文题名: Carbon dioxide dissociation to carbon monoxide by non-thermal plasma
作者: Yap D. ; Tatibouët J.-M. ; Batiot-Dupeyrat C.
刊名: Journal of CO2 Utilization
ISSN: 22129820
出版年: 2015
卷: 12 起始页码: 54
结束页码: 61
语种: 英语
英文关键词: Carbon deposition
; Carbon dioxide activation
; Non-thermal plasma
Scopus关键词: Carbon monoxide
; Dielectric materials
; Dissociation
; Electric discharges
; Electric reactors
; Energy efficiency
; Silica
; Temperature
; AC power supplies
; Carbon deposition
; Carbon dioxide activation
; Low temperatures
; Nonthermal plasma
; Pulsed excitation
; Silica networks
; Sinusoidal excitations
; Carbon dioxide
英文摘要: The decomposition of carbon dioxide was investigated in a non-thermal plasma dielectric barrier discharge reactor filled with glass balls. The CO2 conversion was maximum by using a sinusoidal excitation compared to pulsed excitation. The CO2 conversion and the CO selectivity are increased in the presence of helium, particularly with the AC power supply, but with a decrease in energy efficiency. The formation of solid materials composed of carbon but also of silica was highlighted for the first time, proving that carbon was incorporated into the silica network along with CO2 dissociation under non-thermal plasma conditions. The temperature control of the reactor wall has shown that the CO selectivity is favored by a low temperature wall, whereas the CO2 conversion remained constant, suggesting that the carbon balance default is due to the CO decomposition on the reactor wall. © 2015 Elsevier Ltd. Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/52942
Appears in Collections: 影响、适应和脆弱性
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Recommended Citation:
Yap D.,Tatibouët J.-M.,Batiot-Dupeyrat C.. Carbon dioxide dissociation to carbon monoxide by non-thermal plasma[J]. Journal of CO2 Utilization,2015-01-01,12