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Regional aeromagnetic data from the south-central Zimbabwe Craton have been digitally processed and enhanced for geological and structural mapping and tectonic interpretation integrated with gravity data, to constrain previous interpretations based on tentative geologic maps and provide new information to link these structural features to known tectonic events. The derived maps show excellent correlation between magnetic anomalies and the known geology, and extend lithological and structural mapping to the shallow/near subsurface. In particular, they reveal the presence of discrete crustal domains and several previously unrecognised dykes, faults, and ultramafic intrusions, as well as extensions to others. Five regional structural directions (ENE, NNE, NNW, NW, and WNW) are identified and associated with trends of geological units and cross-cutting structures. The magnetic lineament patterns cut across the >2.7 Ga greenstone belts, which are shown by gravity data to be restricted to the uppermost 10 km of the crust. Therefore, the greenstone belts were an integral part of the lithosphere before much of the upper crustal (brittle) deformation occurred. Significantly, the observed magnetic trends have representatives craton-wide, implying that our interpretation and inferences can be applied to the rest of the craton with confidence. Geological–tectonic correlation suggests that the interpreted regional trends are mainly 2.5 Ga (Great Dyke age) and younger, and relate to tectonic events including the reactivation of the Limpopo Belt at 2.0 Ga and the major regional igneous/dyking events at 1.8–2.0 Ga (Mashonaland), 1.1 Ga (Umkondo), and 180 Ma (Karoo). Thus, their origin is here inferred to be inter- and intra-cratonic collisions and block movements involving the Zimbabwe and Kaapvaal Cratons and the Limpopo Belt, and later lithospheric heating and extension associated with the break-up of Gondwana. The movements produced structures, or reactivated older fractures, that were exploited by Late Archaean and Proterozoic mafic intrusions. There was interplay between vertical and horizontal tectonics as seen in similar terrains worldwide. © 2015, Springer-Verlag Berlin Heidelberg.