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The southwestern flank of the Hellenic fold and thrust belt, situated along the southern edge of the Dinarides–Albanides–Hellenides continental convergent zone, was examined for reconstructing the tectonic deformation. This investigation presents an integrated study of onshore sedimentological and structural analyses, as well as offshore seismic lines, across the Pliocene–Pleistocene sedimentary succession in Zakynthos Island. Back-thrust faults, using the Triassic evaporites as decollement surface, during the Pliocene, and coeval diapiric intrusions formed three sub-basins on the hangingwall of the Kalamaki back-thrust fault. This interaction is responsible for the growth of the Skopos Mountain and the soft sediment deformation that formed synclines and slumps, respectively. Back-thrust and strike-slip faults were active during the early Pleistocene, and diapiric intrusions modified the bathymetry on the sea floor, giving rise to slumps and recumbent folds. At least five events of synsedimentary diapiric intrusions have been recognized and are marked by five slump horizons. During the Holocene, the diapiric intrusions between the Kalamaki back-thrust and the Vrachionas anticline could be either related to normal faults or gravitationally driven. © 2016, Springer-Verlag Berlin Heidelberg.