DOI: 10.1016/j.atmosenv.2014.10.001
Scopus记录号: 2-s2.0-84907995533
论文题名: Twenty years of continuous high time resolution volatile organic compound monitoring in the United Kingdom from 1993 to 2012
作者: Derwent R ; G ; , Dernie J ; I ; R ; , Dollard G ; J ; , Dumitrean P ; , Mitchell R ; F ; , Murrells T ; P ; , Telling S ; P ; , Field R ; A
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2014
卷: 99 起始页码: 239
结束页码: 247
语种: 英语
英文关键词: Hydrocarbons
; Monitoring
; VOC emission inventories
; VOCs
Scopus关键词: Monitoring
; High-time resolution
; United kingdom
; VOC emissions
; VOCs
; Hydrocarbons
; alkane
; alkene derivative
; alkyne derivative
; aromatic hydrocarbon
; hydrocarbon
; isoprene
; volatile organic compound
; atmospheric pollution
; background level
; emission inventory
; pollution monitoring
; rural area
; spatiotemporal analysis
; urban area
; volatile organic compound
; air quality standard
; Article
; catalyst
; chemical reaction
; comparative study
; concentration process
; environmental monitoring
; exhaust gas
; measurement precision
; rural area
; time series analysis
; United Kingdom
; urban area
; United Kingdom
Scopus学科分类: Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要: Continuous, high frequency observations of C2 - C8 hydrocarbons began in the United Kingdom in 1993 and have continued through to the present day at a range of kerbside, urban background and rural locations. Most of the monitored hydrocarbons have shown dramatic declines in concentrations over the study period, with present levels close to an order of magnitude below their levels in the 1990s. The concentrations of 23 selected hydrocarbons have been aggregated up to give an estimate of the total VOC concentrations. These annual values have shown an exponential decline of-18% yr-1 at the London Marylebone Road kerbside site,-11% yr-1 at the London Eltham urban background site and-22% yr-1 at the rural Harwell site. Similar declines have been reported in UK road transport VOC emissions, demonstrating how the VOC emission inventories have apparently captured the salient features influencing real-world VOC emissions over the 1994-2012 period. © 2014 Elsevier Ltd.
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/80567
Appears in Collections: 气候变化事实与影响
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作者单位: Rdscientific, Newbury, United Kingdom; Ricardo-AEA, Gemini Building, Harwell, Oxfordshire, United Kingdom; Department of Atmospheric Science, University of Wyoming, Laramie, WY, United States
Recommended Citation:
Derwent R,G,, Dernie J,et al. Twenty years of continuous high time resolution volatile organic compound monitoring in the United Kingdom from 1993 to 2012[J]. Atmospheric Environment,2014-01-01,99