DOI: 10.1016/j.atmosenv.2013.10.050
Scopus记录号: 2-s2.0-84888347193
论文题名: VOC emissions from residential combustion of Southern and mid-European woods
作者: Evtyugina M ; , Alves C ; , Calvo A ; , Nunes T ; , Tarelho L ; , Duarte M ; , Prozil S ; O ; , Evtuguin D ; V ; , Pio C
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2014
卷: 83 起始页码: 90
结束页码: 98
语种: 英语
英文关键词: Emission factors
; Residential wood combustion
; VOCs
Scopus关键词: Air quality
; Carbon dioxide
; Carbon monoxide
; Chimneys
; Gas chromatography
; Housing
; Hydrocarbons
; Volatile organic compounds
; Wood
; Aliphatic hydrocarbons
; Emission factors
; Operating condition
; Oxygenated compounds
; Residential combustion
; Residential wood combustions
; Tropospheric ozone
; VOCs
; Combustion
; aliphatic hydrocarbon
; benzene
; biofuel
; carbon monoxide
; hemicellulose
; volatile organic compound
; air quality
; biofuel
; biogenic emission
; biomass burning
; carbon dioxide
; carbon emission
; carbon monoxide
; combustion
; desorption
; fuelwood
; gas chromatography
; ozone
; residential energy
; troposphere
; volatile organic compound
; article
; beech
; combustion
; desorption
; gas chromatography
; oak
; Populus
; priority journal
; residential area
; Southern Europe
; wood
; Air Quality
; Carbon Dioxide
; Carbon Monoxide
; Chimneys
; Combustion
; Gas Chromatography
; Hydrocarbons
; Voc
; Wood
; Europe
; Fagus
; Fagus sylvatica
; Populus nigra
Scopus学科分类: Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要: Emissions of trace gases (carbon dioxide (CO2), carbon monoxide (CO), total hydrocarbons (THC)), and volatile organic compounds (VOCs) from combustion of European beech, Pyrenean oak and black poplar in a domestic woodstove and fireplace were studied. These woods are widely used as biofuel in residential combustion in Southern and mid-European countries. VOCs in the flue gases were collected in Tedlar bags, concentrated in sorbent tubes and analysed by thermal desorption-gas chromatography-flame ionisation detection (GC-FID). CO2 emissions ranged from 1415±136 to 1879±29gkg-1 (dry basis). The highest emission factors for CO and THC, 115.8±11.7 and 95.6 24.7±6.3gkg-1 (dry basis), respectively, were obtained during the combustion of black poplar in the fireplace. European beech presented the lowest CO and THC emission factors for both burning appliances. Significant differences in emissions of VOCs were observed among wood species burnt and combustion devices. In general the highest emission factors were obtained from the combustion of Pyrenean oak in the woodstove. Among the VOCs identified, benzene and related compounds were always the most abundant group, followed by oxygenated compounds and aliphatic hydrocarbons. The amount and the composition of emitted VOCs were strongly affected by the wood composition, the type of burning device and operating conditions. Emission data obtained in this work are useful for modelling the impact of residential wood combustion on air quality and tropospheric ozone formation. •Emissions from fireplace and woodstove combustion of three woods were studied.•Woodstove combustion of oak presented the highest emissions among all experiments.•Beech presented the lowest emissions from combustion in both equipments.•Identified VOC emissions were dominated by aromatic compounds for all tested woods.•Emissions are influenced by fuel type, burning appliance and operating conditions. © 2013 Elsevier Ltd. Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/81172
Appears in Collections: 气候变化事实与影响
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作者单位: Centre for Environmental and Marine Studies (CESAM), Department of Environment, University of Aveiro, 3810-193 Aveiro, Portugal; Centre for Research in Ceramic and oComposite Materials (CICECO), Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal
Recommended Citation:
Evtyugina M,, Alves C,, Calvo A,et al. VOC emissions from residential combustion of Southern and mid-European woods[J]. Atmospheric Environment,2014-01-01,83