globalchange  > 气候变化事实与影响
DOI: 10.1016/j.atmosenv.2015.02.034
Scopus记录号: 2-s2.0-84938146004
论文题名:
Assessment of the MACC reanalysis and its influence as chemical boundary conditions for regional air quality modeling in AQMEII-2
作者: Giordano L; , Brunner D; , Flemming J; , Hogrefe C; , Im U; , Bianconi R; , Badia A; , Balzarini A; , Baró R; , Chemel C; , Curci G; , Forkel R; , Jiménez-Guerrero P; , Hirtl M; , Hodzic A; , Honzak L; , Jorba O; , Knote C; , Kuenen J; J; P; , Makar P; A; , Manders-Groot A; , Neal L; , Pérez J; L; , Pirovano G; , Pouliot G; , San José R; , Savage N; , Schröder W; , Sokhi R; S; , Syrakov D; , Torian A; , Tuccella P; , Werhahn J; , Wolke R; , Yahya K; , Žabkar R; , Zhang Y; , Galmarini S
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2015
卷: 115
起始页码: 371
结束页码: 388
语种: 英语
英文关键词: AQMEII-2 ; Model evaluation ; Online-coupled meteorology-chemistry modeling
Scopus关键词: Air quality ; Boundary conditions ; Chemical analysis ; Meteorology ; Quality assurance ; Social networking (online) ; Sulfur dioxide ; AQMEII-2 ; Background concentration ; Chemistry modeling ; Ground based measurement ; Model evaluation ; Regional air quality modeling ; Regional air quality models ; Sensitivity Simulation ; Quality control ; carbon monoxide ; nitrogen ; nitrogen dioxide ; oxide ; ozone ; volatile organic compound ; air quality ; assessment method ; atmospheric modeling ; boundary condition ; concentration (composition) ; ground-based measurement ; numerical model ; oxide ; air quality ; Air Quality Model Evaluation International Initiative ; airport ; Article ; controlled study ; Europe ; North America ; North American ; particulate matter ; priority journal ; secondary organic aerosol ; simulation ; spatial analysis ; summer ; time series analysis ; winter ; Europe ; North America
Scopus学科分类: Environmental Science: Water Science and Technology ; Earth and Planetary Sciences: Earth-Surface Processes ; Environmental Science: Environmental Chemistry
英文摘要: The Air Quality Model Evaluation International Initiative (AQMEII) has now reached its second phase which is dedicated to the evaluation of online coupled chemistry-meteorology models. Sixteen modeling groups from Europe and five from North America have run regional air quality models to simulate the year 2010 over one European and one North American domain. The MACC re-analysis has been used as chemical initial (IC) and boundary conditions (BC) by all participating regional models in AQMEII-2. The aim of the present work is to evaluate the MACC re-analysis along with the participating regional models against a set of ground-based measurements (O3, CO, NO, NO2, SO2, SO42-) and vertical profiles (O3 and CO). Results indicate different degrees of agreement between the measurements and the MACC re-analysis, with an overall better performance over the North American domain. The influence of BC on regional air quality simulations is analyzed in a qualitative way by contrasting model performance for the MACC re-analysis with that for the regional models. This approach complements more quantitative approaches documented in the literature that often have involved sensitivity simulations but typically were limited to only one or only a few regional scale models. Results suggest an important influence of the BC on ozone for which the underestimation in winter in the MACC re-analysis is mimicked by the regional models. For CO, it is found that background concentrations near the domain boundaries are rather close to observations while those over the interior of the two continents are underpredicted by both MACC and the regional models over Europe but only by MACC over North America. This indicates that emission differences between the MACC re-analysis and the regional models can have a profound impact on model performance and points to the need for harmonization of inputs in future linked global/regional modeling studies. © 2015 The Authors.
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/81655
Appears in Collections:气候变化事实与影响

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作者单位: Laboratory for Air Pollution and Environmental Technology, EMPA, Duebendorf, Switzerland; ECMWF, Shinfield Park, Reading, United Kingdom; Atmospheric Modelling and Analysis Division, Environmental Protection Agency, Research Triangle Park, United States; Institute for Environment and Sustainability, Joint Research Centre, European Commission, Ispra, Italy; Enviroware Srl, Concorezzo, MB, Italy; Earth Sciences Department, Barcelona Supercomputing Center (BSC-CNS), Barcelona, Spain; RSE S.p.A., Milano, Italy; University of Murcia, Department of Physics, Physics of the Earth, Ed. CIOyN, Campus de Espinardo, Murcia, Spain; Centre for Atmospheric and Instrumentation Research, University of Hertfordshire, College Lane, Hatfield, United Kingdom; Department of Physical and Chemical Sciences, Center of Excellence for the forecast of Severe Weather (CETEMPS), University of L'Aquila, L'Aquila, Italy; Karlsruher Institut für Technologie (KIT), IMK-IFU, Kreuzeckbahnstr. 19, Garmisch-Partenkirchen, Germany; Section Environmental Meteorology, Division Customer Service, ZAMG - Zentralanstalt fuer Meteorologie und Geodynamik, Wien, Austria; National Center for Atmospheric Research, Boulder, CO, United States; Center of Excellence SPACE-SI, Ljubljana, Slovenia; Netherlands Organization for Applied Scientific Research (TNO), Utrecht, Netherlands; Air Quality Research Section, Atmospheric Science and Technology Directorate, Environment Canada, 4905 Dufferin Street, Toronto, ON, Canada; Met Office, FitzRoy Road, Exeter, United Kingdom; Environmental Software and Modelling Group, Computer Science School - Technical University of Madrid, Campus de Montegancedo - Boadilla del Monte, Madrid, Spain; Atmospheric Modeling and Analysis Division, MD E243-04, U.S. Environmental Protection Agency, Research Triangle Park, NC, United States; Leibniz Institute for Tropospheric Research, Permoserstr. 15, Leipzig, Germany; National Institute of Meteorology and Hydrology, Bulgarian Academy of Sciences, Sofia, Bulgaria; Department of Marine, Earth and Atmospheric Sciences, North Carolina State University, 2800 Faucette Drive, Jordan Hall, Campus Box 8208, United States; University of Ljubljana, Faculty of Mathematics and Physics, Ljubljana, Slovenia; Aarhus University, Department of Environmental Science, Frederiksborgvej 399, Roskilde, Denmark

Recommended Citation:
Giordano L,, Brunner D,, Flemming J,et al. Assessment of the MACC reanalysis and its influence as chemical boundary conditions for regional air quality modeling in AQMEII-2[J]. Atmospheric Environment,2015-01-01,115
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