globalchange  > 气候变化事实与影响
DOI: 10.1016/j.atmosenv.2017.03.047
Scopus记录号: 2-s2.0-85016604380
论文题名:
Photo-chemical transport modelling of tropospheric ozone: A review
作者: Sharma S; , Sharma P; , Khare M
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2017
卷: 159
起始页码: 34
结束页码: 54
语种: 英语
英文关键词: Ozone ; Performance ; Photo-chemical transport modelling ; Resolution
Scopus关键词: Chemical analysis ; Global warming ; Modal analysis ; Optical resolving power ; Productivity ; Sensitivity analysis ; Agricultural productivity ; Chemical transport ; Chemical transport models ; Ozone concentration ; Performance ; Predictive capabilities ; Simulation and modelling ; Tropospheric ozone ; Ozone ; nitrogen oxide ; ozone ; accuracy assessment ; concentration (composition) ; global warming ; literature review ; ozone ; performance assessment ; photochemistry ; pollutant transport ; pollution monitoring ; resolution ; sensitivity analysis ; troposphere ; urban region ; volatile organic compound ; advection ; air pollution ; air pollution control ; air quality ; ambient air ; Asia ; climate change ; dry deposition ; Europe ; global change ; meteorology ; North America ; photochemistry ; physical chemistry ; plume ; pollutant ; priority journal ; radiative forcing ; Review ; sensitivity analysis ; simulation ; solar radiation ; summer ; thermodynamics ; titrimetry ; troposphere ; urban area ; winter
Scopus学科分类: Environmental Science: Water Science and Technology ; Earth and Planetary Sciences: Earth-Surface Processes ; Environmental Science: Environmental Chemistry
英文摘要: Ground level ozone (GLO), a secondary pollutant having adverse impact on human health, ecology, and agricultural productivity, apart from being a major contributor to global warming, has been a subject matter of several studies. In order to identify appropriate strategies to control GLO levels, accurate assessment and prediction is essential, for which elaborate simulation and modelling is required. Several studies have been undertaken in the past to simulate GLO levels at different scales and for various applications. It is important to evaluate these studies, widely spread over in literature. This paper aims to critically review various studies that have been undertaken, especially in the past 15 years (2000–15) to model GLO. The review has been done of the studies that range over different spatial scales – urban to regional and continental to global. It also includes a review of performance evaluation and sensitivity analysis of photo-chemical transport models in order to assess the extent of application of these models and their predictive capability. The review indicates following major findings: (a) models tend to over-estimate the night-time GLO concentrations due to limited titration of GLO with NO within the model; (b) dominance of contribution from far-off regional sources to average ozone concentration in the urban region and higher contribution of local sources during days of high ozone episodes; requiring strategies for controlling precursor emissions at both regional and local scales; (c) greater influence of NOx over VOC in export of ozone from urban regions due to shifting of urban plumes from VOC-sensitive regime to NOx-sensitive as they move out from city centres to neighbouring rural regions; (d) models with finer resolution inputs perform better to a certain extent, however, further improvement in resolutions (beyond 10�km) did not show improvement always; (e) future projections show an increase in GLO concentrations mainly due to rise in temperatures and biogenic VOC emissions. � 2017 Elsevier Ltd
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/82465
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作者单位: Centre for Environmental Studies, The Energy and Resources InstituteNew Delhi, India; Natural Resource and Management Department, Teri UniversityNew Delhi, India; Civil Engineering Department, Indian Institute of TechnologyNew Delhi, India

Recommended Citation:
Sharma S,, Sharma P,, Khare M. Photo-chemical transport modelling of tropospheric ozone: A review[J]. Atmospheric Environment,2017-01-01,159
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