globalchange  > 影响、适应和脆弱性
项目编号: 1506691
项目名称:
Laboratory Studies of Contact Efflorescence
作者: Margaret Tolbert
承担单位: University of Colorado at Boulder
批准年: 2014
开始日期: 2015-08-15
结束日期: 2018-07-31
资助金额: USD438404
资助来源: US-NSF
项目类别: Standard Grant
国家: US
语种: 英语
特色学科分类: Geosciences - Atmospheric and Geospace Sciences
英文关键词: further study contact efflorescence ; efflorescence relative humidity ; immersion efflorescence ; efflorescence mechanism ; laboratory investigation
英文摘要: As atmospheric relative humidity cycles, saline aerosols exist either as ionic salts, or as aqueous ionic solution. Supersaturated and undersaturated phase change typically demonstrate hysteresis behavior as a function of relative humidity. The (increasing) RH at which the phase transition abruptly changes from solid particle to a saturated aqueous solution is the deliquescence relative humidity (DRH). The decreasing RH that drying aqueous droplets remain as supersaturated sols until crystallization, is the efflorescence relative humidity (ERH). Efflorescence may differ based on the nucleation mechanism, either by contact with a seed, or immersion of that seed into the supersaturated droplet. The objective of a series of laboratory investigations is to further study contact efflorescence compared to immersion efflorescence on aerosol types and sizes representative of atmospheric particles. Aerosol phase changes in a single droplet optical trap will be used to systematically follow efflorescence mechanisms.

The importance of accounting for aerosol particle phase changes includes effects on heterogeneous chemical processes, light scattering, and cloud formation and precipitation. Direct effects on homogeneous (gas phase) chemistry and climate also remain uncertain.
资源类型: 项目
标识符: http://119.78.100.158/handle/2HF3EXSE/93702
Appears in Collections:影响、适应和脆弱性
气候减缓与适应

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Margaret Tolbert. Laboratory Studies of Contact Efflorescence. 2014-01-01.
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