globalchange  > 全球变化的国际研究计划
DOI: 10.1021/acs.est.9b02131
WOS记录号: WOS:000484644500029
论文题名:
Simulating and Quantifying Multiple Natural Subsea CO2 Seeps at Panarea Island (Aeolian Islands, Italy) as a Proxy for Potential Leakage from Subseabed Carbon Storage Sites
作者: Gros, Jonas1; Schmidt, Mark1; Dale, Andrew W.1; Linke, Peter1; Vielstadte, Lisa1; Bigalke, Nikolaus1,2; Haeckel, Matthias1; Wallmann, Klaus1; Sommer, Stefan1
通讯作者: Gros, Jonas
刊名: ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN: 0013-936X
EISSN: 1520-5851
出版年: 2019
卷: 53, 期:17, 页码:10258-10268
语种: 英语
WOS关键词: QICS FIELD EXPERIMENT ; NORTH-SEA ; OCEAN ACIDIFICATION ; BUBBLE PLUMES ; WATER COLUMN ; DEEP-SEA ; METHANE ; DYNAMICS ; RELEASE ; DISSOLUTION
WOS学科分类: Engineering, Environmental ; Environmental Sciences
WOS研究方向: Engineering ; Environmental Sciences & Ecology
英文摘要:

Carbon dioxide (CO2) capture and storage (CCS) has been discussed as a potentially significant mitigation option for the ongoing climate warming. Natural CO2 release sites serve as natural laboratories to study subsea CO2 leakage in order to identify suitable analytical methods and numerical models to develop best-practice procedures for the monitoring of subseabed storage sites. We present a new model of bubble (plume) dynamics, advection-dispersion of dissolved CO2, and carbonate chemistry. The focus is on a medium-sized CO2 release from 294 identified small point sources around Panarea Island (South-East Tyrrhenian Sea, Aeolian Islands, Italy) in water depths of about 40-50 m. This study evaluates how multiple CO2 seep sites generate a temporally variable plume of dissolved CO2. The model also allows the overall flow rate of CO2 to be estimated based on field measurements of pH. Simulations indicate a release of similar to 6900 t y(-1) of CO2 for the investigated area and highlight an important role of seeps located at >20 m water depth in the carbon budget of the Panarea offshore gas release system. This new transport-reaction model provides a framework for understanding potential future leaks from CO2 storage sites.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/146722
Appears in Collections:全球变化的国际研究计划

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作者单位: 1.GEOMAR Helmholtz Ctr Ocean Res Kiel, RD2 Marine Geosyst Wischhofstr 1-3, D-24148 Kiel, Germany
2.Geotek, 3 Faraday Close, Daventry NN11 8RD, Northants, England

Recommended Citation:
Gros, Jonas,Schmidt, Mark,Dale, Andrew W.,et al. Simulating and Quantifying Multiple Natural Subsea CO2 Seeps at Panarea Island (Aeolian Islands, Italy) as a Proxy for Potential Leakage from Subseabed Carbon Storage Sites[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2019-01-01,53(17):10258-10268
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